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Abstract
A long-term goal for superconductors is to increase the superconducting transition temperature, T C . In cuprates, T C depends strongly on the out-of-plane Cu-apical oxygen distance and the in-plane Cu-O distance, but there has been little attention paid to tuning them independently. Here, in simply grown, self-assembled, vertically aligned nanocomposite thin films of La 2 CuO 4+δ + LaCuO 3 , by strongly increasing out-of-plane distances without reducing in-plane distances (three-dimensional strain engineering), we achieve superconductivity up to 50 K in the vertical interface regions, spaced ~50 nm apart. No additional process to supply excess oxygen, e.g., by ozone or high-pressure oxygen annealing, was required, as is normally the case for plain La 2 CuO 4+δ films. Finally, our proof-of-concept work represents an entirely new approach to increasing >T C n cuprates or other superconductors.