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http://hdl.handle.net/10251/153692

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Influence of co-catalysts on the photocatalytic activity of MIL-125(Ti)-NH2 in the overall water splitting

Abstract

[EN] Titanium containing aminoterephthalate metal organic framework promotes the photocatalytic overall water splitting into H-2 and O-2 at a rate that depends on the presence of Pt, RuOx and CoOx co-catalyst. The best values of have been obtained for the MIL-125-NH2 material that contains Pt and RuOx, reaching a production of 218 and 85 mu mol/g (-1)(photocataly)(st) at 24 h for H-2 and O-2, respectively. Financial support by the Spanish Ministry of Economy and Competitiveness [Severo Ochoa and CTQ2015-69163-CO2-R1] and Generalitat Valenciana [Prometeo 2017-083] is gratefully acknowledged. S.R.-B. also thanks the Research Executive Agency (REA) and the European Commission, for the funding received under the Marie Sklodowska-Curie actions [H2020-MSCA-IF-2015/ Grant agreement number 709023/ ZESMO]. S.N. thanks financial support by the Fundacion Ramon Areces (XVIII Concurso Nacional para la Adjudicacion de Ayudas a la Investigacion en Ciencias de la Vida y de la Materia, 2016). The authors also wish to acknowledge the support provided by the Electron Microscopy Service facility at Universitat Politecnica de Valencia. Remiro-Buenamañana, S.; Cabrero-Antonino, M.; Martínez-Guanter, M.; Alvaro Rodríguez, MM.; Navalón Oltra, S.; García Gómez, H. (2019). Influence of co-catalysts on the photocatalytic activity of MIL-125(Ti)-NH2 in the overall water splitting. Applied Catalysis B Environmental. 254:677-684. https://doi.org/10.1016/j.apcatb.2019.05.027

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